Sea spray as a secondary source of chlorinated persistent organic pollutants? - Conclusions from a comparison of seven fresh snowfall events in 2019 and 2021 - Publikacja - MOST Wiedzy

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Sea spray as a secondary source of chlorinated persistent organic pollutants? - Conclusions from a comparison of seven fresh snowfall events in 2019 and 2021

Abstrakt

Secondary sources of persistent organic pollutants (POPs) gain in importance worldwide as primary sources decline. In this work, we aim to determine whether sea spray may be a secondary source of chlorinated POPs to the terrestrial Arctic, since a similar mechanism was proposed there only for the more water-soluble POPs. To this end, we have determined polychlorinated biphenyls and organochlorine pesticides concentrations in fresh snow and seawater collected in the vicinity of the Polish Polar Station in Hornsund in two sampling periods covering spring 2019 and 2021. To support our interpretations, we include also metal and metalloid, and stable hydrogen and oxygen isotopes analysis in those samples. A significant correlation was found between the concentrations of POPs and the distance from the sea at the sampling point, yet the confirmation of sea spray impact lies more in capturing an event with negligible long-range transport influence where the detected chlorinated POPs (Cl-POPs) matched in composition the compounds enriched in the sea surface microlayer, which is both a source of sea spray and a seawater microenvironment rich in hydrophobic substances.

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Accepted albo Published Version
DOI:
Cyfrowy identyfikator dokumentu elektronicznego (otwiera się w nowej karcie) 10.1016/j.scitotenv.2023.164357
Licencja
Creative Commons: CC-BY otwiera się w nowej karcie

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Informacje szczegółowe

Kategoria:
Publikacja w czasopiśmie
Typ:
artykuły w czasopismach
Opublikowano w:
SCIENCE OF THE TOTAL ENVIRONMENT nr 891,
ISSN: 0048-9697
Język:
angielski
Rok wydania:
2023
Opis bibliograficzny:
Pawlak F., Koziol K., Frankowski M., Nowicki Ł., Marlin C., Sulej-Suchomska A. M., Polkowska Ż.: Sea spray as a secondary source of chlorinated persistent organic pollutants? - Conclusions from a comparison of seven fresh snowfall events in 2019 and 2021// SCIENCE OF THE TOTAL ENVIRONMENT -,iss. 891 (2023), s.164357-
DOI:
Cyfrowy identyfikator dokumentu elektronicznego (otwiera się w nowej karcie) 10.1016/j.scitotenv.2023.164357
Źródła finansowania:
  • IDUB
Weryfikacja:
Politechnika Gdańska

wyświetlono 79 razy

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