Search
Carbon nitride exfoliation for photocatalysis and photocatalytic ozonation over emerging contaminants abatement
Abstract
The production of graphitic carbon nitride was studied with the addition of a following exfoliation step using ultrasounds, at different times. The treatment produced catalysts with much higher surface areas, from 2.18 m2 g 1 with no treatment to 28.34 m2 g 1 after 36 h of exfoliation. During exfoliation, melem was also produced, and may further enhance the photoluminescence and photocatalytic properties. The photocatalytic reaction also indicated the improved performance of exfoliated g-C3N4 towards the degradation of a mixture of parabens, enhancing their removal from 20% to up to 65% in 2 h under UVA radiation. The combination of ozone and g- C3N4 photocatalysis was able to completely remove the parabens in under 8 min and with a 20% lower consumption of ozone compared to photolytic ozonation. The main reactive species were identified, and the byproducts formed during parabens degradation were detected. The efficiency of the combined system was also attested by using a mixture of parabens and other common drugs, maintaining its better performance.
Citations
-
6
CrossRef
-
0
Web of Science
-
6
Scopus
Authors (8)
-
Eryk Fernandes
-
Paweł Mazierski dr inż.
-
Magdalena Miodyńska
-
Mirosława Pawlyta
-
Adriana Zaleska-Medynska Prof. dr hab. inż.
-
Rui F. Martins
-
João Gomes
Cite as
Full text
- Publication version
- Accepted or Published Version
- DOI:
- Digital Object Identifier (open in new tab) 10.1016/j.jece.2023.110554
- License
-
open in new tab
Keywords
Details
- Category:
- Articles
- Type:
- artykuły w czasopismach
- Published in:
-
Journal of Environmental Chemical Engineering
no. 11,
ISSN: 2213-2929 - Language:
- English
- Publication year:
- 2023
- Bibliographic description:
- Fernandes E., Mazierski P., Miodyńska M., Klimczuk T., Pawlyta M., Zaleska-Medynska A., Martins R. F., Gomes J.: Carbon nitride exfoliation for photocatalysis and photocatalytic ozonation over emerging contaminants abatement// Journal of Environmental Chemical Engineering -Vol. 11,iss. 5 (2023), s.110554-
- DOI:
- Digital Object Identifier (open in new tab) 10.1016/j.jece.2023.110554
- Sources of funding:
-
- Free publication
- Verified by:
- Gdańsk University of Technology
seen 43 times
Recommended for you
g-C3N4 for Photocatalytic Degradation of Parabens: Precursors Influence, the Radiation Source and Simultaneous Ozonation Evaluation
- E. Fernandes,
- P. Mazierski,
- T. Klimczuk
- + 3 authors
The role of noble metals in TiO2 nanotubes for the abatement of parabens by photocatalysis, catalytic and photocatalytic ozonation
- J. Lincho,
- E. Domingues,
- P. Mazierski
- + 5 authors
TiO2 nanotube arrays-based reactor for photocatalytic oxidation of parabens mixtures in ultrapure water: Effects of photocatalyst properties, operational parameters and light source
- J. Gomes,
- J. Lincho,
- M. Domingues
- + 7 authors