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High-performance NdSrCo2O5+δ–Ce0.8Gd0.2O2-δ composite cathodes for electrolyte-supported microtubular solid oxide fuel cells
Abstrakt
NdSrCo2O5+δ (NSCO) is a perovskite with an electrical conductivity of 1551.3 S cm−1 at 500 °C and 921.7 S cm−1 at 800 °C and has a metal-like temperature dependence. This perovskite is used as the cathode material for Ce0.8Gd0.2O2-δ (GDC)-supported microtubular solid oxide fuel cells (MT-SOFCs). The MT-SOFCs fabricated in this study consist of a bilayer anode, comprising a NiO–GDC composite layer and a NiO layer, and a NSCO–GDC composite cathode. Three cell designs with different outer tube diameters, GDC thicknesses, and NSCO/GDC ratios are designed. The MT-SOFC with an outer tube diameter of 1.86 mm, an electrolyte thickness of 180 μm, and a 5NSCO–5GDC composite cathode presents the best performance. The flexural strength of the aforementioned cell is 177 MPa, which is sufficient to confer mechanical integrity to the cell. Moreover, the ohmic and polarization resistance values of the cell are 0.22 and 0.09 Ω cm2 at 700 °C, respectively, and 0.15 and 0.03 Ω cm2 at 800 °C, respectively. These results indicate that the NSCO-GDC composite exhibits high electrochemical activity. The maximum power densities of the cell at 700 and 800 °C are 0.46 and 0.67 W cm−2, respectively, exceeding those of existing electrolyte-supported MT-SOFCs with similar electrolyte thicknesses.
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Autorzy (5)
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Sea-Fue Wang
- National Taipei University of Technology
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Yung-Fu Hsu
- National Taipei University of Technology
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Yi-Le Liao
- National Taipei University of Technology
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Shih-Ting Huang
- National Taipei University of Technology
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Informacje szczegółowe
- Kategoria:
- Publikacja w czasopiśmie
- Typ:
- artykuły w czasopismach
- Opublikowano w:
-
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
nr 46,
strony 31778 - 31787,
ISSN: 0360-3199 - Język:
- angielski
- Rok wydania:
- 2021
- Opis bibliograficzny:
- Wang S., Hsu Y., Liao Y., Huang S., Jasiński P.: High-performance NdSrCo2O5+δ–Ce0.8Gd0.2O2-δ composite cathodes for electrolyte-supported microtubular solid oxide fuel cells// INTERNATIONAL JOURNAL OF HYDROGEN ENERGY -Vol. 46,iss. 62 (2021), s.31778-31787
- DOI:
- Cyfrowy identyfikator dokumentu elektronicznego (otwiera się w nowej karcie) 10.1016/j.ijhydene.2021.07.049
- Weryfikacja:
- Politechnika Gdańska
wyświetlono 118 razy
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