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Structural and electrochemical heterogeneities of boron-doped diamond surfaces

Abstract

This brief review is focussed on the recent progress in studies of the heterogeneous electrochemical behaviour of various boron-doped materials extending from zero-dimensional particles through polycrystalline or nanostructured three-dimensional surfaces. A boron-doped diamond reveals large heterogeneities induced by numerous factors, inter alia multi-faceted crystallinity, inhomogeneous boron concentration, sp2/sp3-carbon ratio, surface terminations and grain size distribution. We also present single nanodiamond particles and a nanostructured diamond, which are fabricated by either a top-down or a bottom-up procedure. Nanoarchitectured surfaces allow high areas and large aspect ratios to be achieved, exhibiting highly heterogeneous charge-transfer performance for catalytic, sensing and energy applications. We have anticipated multi-factor-originated heterogeneities of various boron-doped diamond surfaces displaying the essential fabrication and diagnostic methodologies and critically reviewing their benefits and drawbacks.

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DOI:
Digital Object Identifier (open in new tab) 10.1016/j.coelec.2021.100876
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Details

Category:
Articles
Type:
artykuły w czasopismach
Published in:
Current Opinion in Electrochemistry no. 31,
ISSN: 2451-9103
Language:
English
Publication year:
2022
Bibliographic description:
Bogdanowicz S., Ryl J.: Structural and electrochemical heterogeneities of boron-doped diamond surfaces// Current Opinion in Electrochemistry -, (2021), s.100876-
DOI:
Digital Object Identifier (open in new tab) 10.1016/j.coelec.2021.100876
Sources of funding:
Verified by:
Gdańsk University of Technology

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