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Detailed investigation of the phase transition inKxP4W8O32and experimental arguments for a charge density wave due to hidden nesting

Abstract

Detailed structural and magnetotransport properties of monophosphate tungsten bronze Kx(PO2)4(WO3)8 single crystals are reported. Both galvanomagnetic and thermal properties are shown to be consistent with a charge density wave electronic transition due to hidden nesting of the quasi-1D portion of the Fermi surface. We also observe the enhancement of electronic anisotropy due to reconstruction of the Fermi surface at the Peierls transition. The resistivity presents a thermal hysteresis suggesting a first-order nature characteristic of a strong-coupling scenario. However, other measurements such as the change of carrier density demonstrate a second-order Peierls scenario with weak-coupling features. We suggest that the structural transition driven by the residual strain in the K-P-O environment is responsible for the resistivity hysteresis and modifies the Fermi surface which then helps the rise to the second-order Peierls instability.

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DOI:
Digital Object Identifier (open in new tab) 10.1103/PhysRevB.93.235126
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Copyright (2016 American Physical Society)

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Category:
Articles
Type:
artykuł w czasopiśmie wyróżnionym w JCR
Published in:
PHYSICAL REVIEW B no. 93, pages 1 - 10,
ISSN: 2469-9950
Language:
English
Publication year:
2016
Bibliographic description:
Kolincio K., Pérez O., Hébert S., Fertey P., Pautrat A.: Detailed investigation of the phase transition inKxP4W8O32and experimental arguments for a charge density wave due to hidden nesting// PHYSICAL REVIEW B. -Vol. 93, (2016), s.1-10
DOI:
Digital Object Identifier (open in new tab) 10.1103/physrevb.93.235126
Verified by:
Gdańsk University of Technology

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