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Stripe order and magnetic anisotropy in the S=1 antiferromagnet BaMoP2O8

Abstract

Magnetic behavior of yavapaiite-type BaMoP2O8 with the spatially anisotropic triangular arrangement of the S=1Mo4+ ions is explored using thermodynamic measurements, neutron diffraction, and density-functional band-structure calculations. A broad maximum in the magnetic susceptibility around 46 K is followed by the stripe antiferromagnetic order with the propagation vector k=(12,12,12) formed below TN≃21 K. This stripe phase is triggered by a pronounced one-dimensionality of the spin lattice, where one of the in-plane couplings, J2≃4.6 meV, is much stronger than its J1≃0.4 meV counterpart, and stabilized by the weak easy-axis anisotropy. The ordered moment of 1.42(9)μB at 1.5 K is significantly lower than the spin-only moment of 2μB due to a combined effect of quantum fluctuations and spin-orbit coupling.

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DOI:
Digital Object Identifier (open in new tab) 10.1103/PhysRevB.98.094406
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Copyright (2018 American Physical Society)

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Category:
Articles
Type:
artykuł w czasopiśmie wyróżnionym w JCR
Published in:
PHYSICAL REVIEW B no. 98, edition 9, pages 1 - 9,
ISSN: 2469-9950
Language:
English
Publication year:
2018
Bibliographic description:
Hembacher J., Badrtdinov D., Ding L., Sobczak Z., Ritter C., Mazurenko V., Tsirlin A.: Stripe order and magnetic anisotropy in the S=1 antiferromagnet BaMoP2O8// PHYSICAL REVIEW B. -Vol. 98, iss. 9 (2018), s.1-9
DOI:
Digital Object Identifier (open in new tab) 10.1103/physrevb.98.094406
Verified by:
Gdańsk University of Technology

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